4-(((4-Methoxyphenyl)amino)methyl)-N,N-dimethylaniline and 2-Methoxy-5-((phenylamino)methyl)phenol

Molecular structures of 4-(((4-methoxyphenyl)amino)methyl)-N,N-dimethylaniline and 2-methoxy-5-((phenylamino)methyl)phenol synthesized via Schiff bases reduction route are reported. The compounds consist asymmetric units C16H20N2O (1) C14H15NO2 (2) in orthorhombic monoclinic crystal systems, respectively. Compound 1 intermolecular C11—H11···N2 hydrogen bonding with C11···N21 = 3.463(4) Å. hydroxyl group 2 is also involved O2—H2···O2 O2—H2···O21 O2···O11 2.8885(15) Å O1···O21 2.9277(5) molecular the stabilized by secondary interactions C1—H1B···O11 C5—H···(C41, C51, C61, C71) for H···C, C—H···O N—H···C 2. reported important starting material synthesis many such as azo dyes dithiocarbamate.